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Loly (ロリ, Rori) is the 33rd Arrancar in Sōsuke Aizen's army. She, along with Menoly, were ordered to bring Orihime Inoue to Aizen when he wanted to show her the Hōgyoku. She develops a deep hatred towards the captured Human girl, and clearly has an intention to kill her, even if that means going against Aizen's orders.

She seems infatuated with Aizen, as shown by her anger at Aizen's interest in Orihime. She also seems to be very impulsive and easily-angered, seen when she almost beats Orihime to death after she asked her to leave her room (and Menoly tried to stop her from "taking it too far", but could not stop her).

In the anime, Loly's fate is still the same but given a little more detail. When Yammy hurts her, Loly accuses Orihime of enjoying her suffering, but is shocked as Orihime again heals her wounds. When Yammy attacks Orihime, she defends her, hatefully saying she owes her and the ensuing battle lasts a bit longer, but ends the same way. When she is in Yammy's grasp, Loly shouts at Orihime not to help her, again declaring her hatred towards her. But she gives Orihime a smile before she meets her fate at Yammy's hand. The smile Loly gave Orihime, as well as the act of defending her, may imply that while she still hates Orihime, she might have come to terms with her feelings, or it may simply have been a farwell and returning favor for healing her.